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Make sure controller isn't paired to another device.
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sudo rm -R /Library/Preferences/com.apple.Bluetooth.plist
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Restart
3a. With BT PrefPane open, try pairing with PS Button and Share. May or may not work. If it does, you're done!
3b. If 3a doesn't work, try connecting by pressing PS button and looking to see if light stays lit.
- If still not working, start at step 2, and possibly try only 3b.