diff --git a/.github/workflows/ci-libshortfin.yml b/.github/workflows/ci-libshortfin.yml
index 0e0982803..543a6abe6 100644
--- a/.github/workflows/ci-libshortfin.yml
+++ b/.github/workflows/ci-libshortfin.yml
@@ -38,7 +38,7 @@ jobs:
     strategy:
       fail-fast: false
       matrix:
-        name: ["Ubuntu (Clang)(full)", "Ubuntu (Clang)(host-only)", "Ubuntu (GCC)", "Windows (MSVC)"]
+        name: ["Ubuntu (Clang)(full)", "Ubuntu (Clang)(host-only)", "Windows (MSVC)"]
         python-version: ["3.10", "3.11", "3.12"]
         include:
           - name: Ubuntu (Clang)(full)
@@ -53,16 +53,21 @@ jobs:
             cmake-options:
               -DCMAKE_C_COMPILER=clang-18 -DCMAKE_CXX_COMPILER=clang++-18 -DCMAKE_LINKER_TYPE=LLD -DSHORTFIN_HAVE_AMDGPU=OFF -DSHORTFIN_BUILD_STATIC=ON -DSHORTFIN_BUILD_DYNAMIC=ON
             additional-packages: clang lld
-          - name: Ubuntu (GCC)
+          - name: Ubuntu (GCC 13)
             runs-on: ubuntu-24.04
+            # Only test with GCC 13 and Python 3.12
+            python-version: "3.12"
+            cmake-options:
+              -DCMAKE_C_COMPILER=gcc-13 -DCMAKE_CXX_COMPILER=g++-13
+          - name: Ubuntu (GCC 14)
+            runs-on: ubuntu-24.04
+            # Only test with GCC 14 and Python 3.12
+            python-version: "3.12"
+            cmake-options:
+              -DCMAKE_C_COMPILER=gcc-14 -DCMAKE_CXX_COMPILER=g++-14
           - name: Windows (MSVC)
             runs-on: windows-2022
         exclude:
-          # Only test Python 3.12 with GCC
-          - name: Ubuntu (GCC)
-            python-version: "3.10"
-          - name: Ubuntu (GCC)
-            python-version: "3.11"
           # TODO: Include additional Python versions for Windows after build got fixed
           - name: Windows (MSVC)
             python-version: "3.10"