From 573184cd60b180bfc27ebedaeae554de5656a7c1 Mon Sep 17 00:00:00 2001 From: Jonathan Schmidt <54937397+JonathanSchmidt1@users.noreply.github.com> Date: Thu, 7 Mar 2024 20:37:04 +0100 Subject: [PATCH] Add nequip force field relax- and staticmaker and corresponding tests (#764) * add nequip force field relax- and staticmaker and corresponding tests * fix model_kwargs doc string * change tests to smaller force field * add nequip and torch-runstats to testing.yml for CI * Add nequip and torch-runstats to Install dependencies in deploy.yml * Revert "Add nequip and torch-runstats to Install dependencies in deploy.yml" This reverts commit 7080af553014e51ae36f0a31008ce35b6c24a321. * minor refactor * rename nequip_sto_test_ff.pth to nequip_ff_sr_ti_o3.pth --------- Co-authored-by: Janosh Riebesell --- .github/workflows/testing.yml | 2 + src/atomate2/forcefields/__init__.py | 1 + src/atomate2/forcefields/jobs.py | 92 ++++++++++++++++++ tests/conftest.py | 5 + tests/forcefields/test_jobs.py | 63 +++++++++++- .../forcefields/nequip/nequip_ff_sr_ti_o3.pth | Bin 0 -> 254215 bytes tests/test_data/structures/SrTiO3.cif | 81 +++++++++++++++ 7 files changed, 239 insertions(+), 5 deletions(-) create mode 100644 tests/test_data/forcefields/nequip/nequip_ff_sr_ti_o3.pth create mode 100644 tests/test_data/structures/SrTiO3.cif diff --git a/.github/workflows/testing.yml b/.github/workflows/testing.yml index b91ace2195..e5ed45cbce 100644 --- a/.github/workflows/testing.yml +++ b/.github/workflows/testing.yml @@ -55,6 +55,8 @@ jobs: # ase needed to get FrechetCellFilter used by ML force fields pip install git+https://gitlab.com/ase/ase pip install .[strict,tests] + pip install torch-runstats + pip install --no-deps nequip - name: Test env: diff --git a/src/atomate2/forcefields/__init__.py b/src/atomate2/forcefields/__init__.py index 362ade8980..3e7ac5ac47 100644 --- a/src/atomate2/forcefields/__init__.py +++ b/src/atomate2/forcefields/__init__.py @@ -10,3 +10,4 @@ class MLFF(Enum): # TODO inherit from StrEnum when 3.11+ GAP = "GAP" M3GNet = "M3GNet" CHGNet = "CHGNet" + Nequip = "Nequip" diff --git a/src/atomate2/forcefields/jobs.py b/src/atomate2/forcefields/jobs.py index 047694654c..a92ba652de 100644 --- a/src/atomate2/forcefields/jobs.py +++ b/src/atomate2/forcefields/jobs.py @@ -255,6 +255,98 @@ def _relax(self, structure: Structure) -> dict: return relaxer.relax(structure, steps=self.steps, **self.relax_kwargs) +@dataclass +class NequipRelaxMaker(ForceFieldRelaxMaker): + """ + Maker to perform a relaxation using a Nequip force field. + + Parameters + ---------- + name : str + The job name. + force_field_name : str + The name of the force field. + relax_cell : bool = True + Whether to allow the cell shape/volume to change during relaxation. + steps : int + Maximum number of ionic steps allowed during relaxation. + relax_kwargs : dict + Keyword arguments that will get passed to :obj:`Relaxer.relax`. + optimizer_kwargs : dict + Keyword arguments that will get passed to :obj:`Relaxer()`. + task_document_kwargs : dict + Additional keyword args passed to :obj:`.ForceFieldTaskDocument()`. + model_path: str | Path + deployed model checkpoint to load with + :obj:`nequip.calculators.NequipCalculator.from_deployed_model()'`. + model_kwargs: dict[str, Any] + Further keywords (e.g. device: Union[str, torch.device], + species_to_type_name: Optional[Dict[str, str]] = None) for + :obj:`nequip.calculators.NequipCalculator()'`. + """ + + name: str = f"{MLFF.Nequip} relax" + force_field_name: str = f"{MLFF.Nequip}" + relax_cell: bool = True + steps: int = 500 + relax_kwargs: dict = field(default_factory=dict) + optimizer_kwargs: dict = field(default_factory=dict) + task_document_kwargs: dict = field(default_factory=dict) + model_path: str | Path = "" + model_kwargs: dict = field(default_factory=dict) + + def _relax(self, structure: Structure) -> dict: + from nequip.ase import NequIPCalculator + + calculator = NequIPCalculator.from_deployed_model( + self.model_path, **self.model_kwargs + ) + relaxer = Relaxer( + calculator, relax_cell=self.relax_cell, **self.optimizer_kwargs + ) + + return relaxer.relax(structure, steps=self.steps, **self.relax_kwargs) + + +@dataclass +class NequipStaticMaker(ForceFieldStaticMaker): + """ + Maker to calculate energies, forces and stresses using a nequip force field. + + Parameters + ---------- + name : str + The job name. + force_field_name : str + The name of the force field. + task_document_kwargs : dict + Additional keyword args passed to :obj:`.ForceFieldTaskDocument()`. + model_path: str | Path + deployed model checkpoint to load with + :obj:`nequip.calculators.NequipCalculator()'`. + model_kwargs: dict[str, Any] + Further keywords (e.g. device: Union[str, torch.device], + species_to_type_name: Optional[Dict[str, str]] = None) for + :obj:`nequip.calculators.NequipCalculator()'`. + """ + + name: str = f"{MLFF.Nequip} static" + force_field_name: str = f"{MLFF.Nequip}" + task_document_kwargs: dict = field(default_factory=dict) + model_path: str | Path = "" + model_kwargs: dict = field(default_factory=dict) + + def _evaluate_static(self, structure: Structure) -> dict: + from nequip.ase import NequIPCalculator + + calculator = NequIPCalculator.from_deployed_model( + self.model_path, **self.model_kwargs + ) + relaxer = Relaxer(calculator, relax_cell=False) + + return relaxer.relax(structure, steps=1) + + @dataclass class M3GNetStaticMaker(ForceFieldStaticMaker): """ diff --git a/tests/conftest.py b/tests/conftest.py index 4280e9073b..57c444f504 100644 --- a/tests/conftest.py +++ b/tests/conftest.py @@ -97,6 +97,11 @@ def si_structure(test_dir): return Structure.from_file(test_dir / "structures" / "Si.cif") +@pytest.fixture() +def sr_ti_o3_structure(test_dir): + return Structure.from_file(test_dir / "structures" / "SrTiO3.cif") + + @pytest.fixture(autouse=True) def mock_jobflow_settings(memory_jobstore): """Mock the jobflow settings to use our specific jobstore (with data store).""" diff --git a/tests/forcefields/test_jobs.py b/tests/forcefields/test_jobs.py index e6249486f8..95527bb16c 100644 --- a/tests/forcefields/test_jobs.py +++ b/tests/forcefields/test_jobs.py @@ -2,6 +2,7 @@ import pytest from jobflow import run_locally +from pymatgen.core import Structure from pytest import approx, importorskip from atomate2.forcefields.jobs import ( @@ -13,6 +14,8 @@ M3GNetStaticMaker, MACERelaxMaker, MACEStaticMaker, + NequipRelaxMaker, + NequipStaticMaker, ) from atomate2.forcefields.schemas import ForceFieldTaskDocument @@ -35,7 +38,7 @@ def test_chgnet_static_maker(si_structure): @pytest.mark.parametrize("relax_cell", [True, False]) -def test_chgnet_relax_maker(si_structure, relax_cell: bool): +def test_chgnet_relax_maker(si_structure: Structure, relax_cell: bool): # translate one atom to ensure a small number of relaxation steps are taken si_structure.translate_sites(0, [0, 0, 0.1]) @@ -101,7 +104,7 @@ def test_m3gnet_relax_maker(si_structure): @mace_paths -def test_mace_static_maker(si_structure, test_dir, model): +def test_mace_static_maker(si_structure: Structure, test_dir: Path, model): task_doc_kwargs = {"ionic_step_data": ("structure", "energy")} # generate job @@ -122,7 +125,9 @@ def test_mace_static_maker(si_structure, test_dir, model): @pytest.mark.parametrize("relax_cell", [True, False]) @mace_paths -def test_mace_relax_maker(si_structure, test_dir, model, relax_cell: bool): +def test_mace_relax_maker( + si_structure: Structure, test_dir: Path, model, relax_cell: bool +): # translate one atom to ensure a small number of relaxation steps are taken si_structure.translate_sites(0, [0, 0, 0.1]) @@ -149,7 +154,7 @@ def test_mace_relax_maker(si_structure, test_dir, model, relax_cell: bool): assert output1.output.n_steps == 4 -def test_gap_static_maker(si_structure, test_dir): +def test_gap_static_maker(si_structure: Structure, test_dir): importorskip("quippy") task_doc_kwargs = {"ionic_step_data": ("structure", "energy")} @@ -172,8 +177,56 @@ def test_gap_static_maker(si_structure, test_dir): assert output1.output.n_steps == 1 +def test_nequip_static_maker(sr_ti_o3_structure: Structure, test_dir: Path): + task_doc_kwargs = {"ionic_step_data": ("structure", "energy")} + + # generate job + # NOTE the test model is not trained on Si, so the energy is not accurate + job = NequipStaticMaker( + task_document_kwargs=task_doc_kwargs, + model_path=test_dir / "forcefields" / "nequip" / "nequip_ff_sr_ti_o3.pth", + ).make(sr_ti_o3_structure) + + # run the flow or job and ensure that it finished running successfully + responses = run_locally(job, ensure_success=True) + + # validation the outputs of the job + output1 = responses[job.uuid][1].output + assert isinstance(output1, ForceFieldTaskDocument) + assert output1.output.energy == approx(-44.40017, rel=1e-4) + assert output1.output.n_steps == 1 + + +@pytest.mark.parametrize("relax_cell", [True, False]) +def test_nequip_relax_maker( + sr_ti_o3_structure: Structure, test_dir: Path, relax_cell: bool +): + # translate one atom to ensure a small number of relaxation steps are taken + sr_ti_o3_structure.translate_sites(0, [0, 0, 0.2]) + # generate job + job = NequipRelaxMaker( + steps=25, + optimizer_kwargs={"optimizer": "BFGSLineSearch"}, + relax_cell=relax_cell, + model_path=test_dir / "forcefields" / "nequip" / "nequip_ff_sr_ti_o3.pth", + ).make(sr_ti_o3_structure) + + # run the flow or job and ensure that it finished running successfully + responses = run_locally(job, ensure_success=True) + + # validation the outputs of the job + output1 = responses[job.uuid][1].output + assert isinstance(output1, ForceFieldTaskDocument) + if relax_cell: + assert output1.output.energy == approx(-44.407, rel=1e-3) + assert output1.output.n_steps == 5 + else: + assert output1.output.energy == approx(-44.40015, rel=1e-4) + assert output1.output.n_steps == 5 + + @pytest.mark.parametrize("relax_cell", [True, False]) -def test_gap_relax_maker(si_structure, test_dir, relax_cell: 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