From 0817ede303a3de2d493a2d77ffd16da3a56d14b1 Mon Sep 17 00:00:00 2001 From: Andrey Sobolev Date: Tue, 16 Jul 2024 15:25:53 +0200 Subject: [PATCH] Equation of State workflow for FHI-aims (#889) * Added EOS FHI-aims workflow * Added tmp_path to phonon tests * Added test data for EOS workflow * Tests changed for older Pymatgen version * simplify from_parameters * Change the test reference value --------- Co-authored-by: Janosh Riebesell --- src/atomate2/aims/flows/eos.py | 82 ++++++++++++++ tests/aims/test_flows/test_eos.py | 104 ++++++++++++++++++ tests/aims/test_flows/test_phonon_workflow.py | 4 +- .../aims/eos-si/0/inputs/control.in.gz | Bin 0 -> 1195 bytes .../aims/eos-si/0/inputs/geometry.in.gz | Bin 0 -> 170 bytes .../aims/eos-si/0/outputs/aims.out.gz | Bin 0 -> 20526 bytes .../aims/eos-si/1/inputs/control.in.gz | Bin 0 -> 1195 bytes .../aims/eos-si/1/inputs/geometry.in.gz | Bin 0 -> 177 bytes .../aims/eos-si/1/outputs/aims.out.gz | Bin 0 -> 20483 bytes .../aims/eos-si/2/inputs/control.in.gz | Bin 0 -> 1195 bytes .../aims/eos-si/2/inputs/geometry.in.gz | Bin 0 -> 174 bytes .../aims/eos-si/2/outputs/aims.out.gz | Bin 0 -> 20306 bytes .../aims/eos-si/3/inputs/control.in.gz | Bin 0 -> 1195 bytes .../aims/eos-si/3/inputs/geometry.in.gz | Bin 0 -> 169 bytes .../aims/eos-si/3/outputs/aims.out.gz | Bin 0 -> 20438 bytes 15 files changed, 188 insertions(+), 2 deletions(-) create mode 100644 src/atomate2/aims/flows/eos.py create mode 100644 tests/aims/test_flows/test_eos.py create mode 100644 tests/test_data/aims/eos-si/0/inputs/control.in.gz create mode 100644 tests/test_data/aims/eos-si/0/inputs/geometry.in.gz create mode 100644 tests/test_data/aims/eos-si/0/outputs/aims.out.gz create mode 100644 tests/test_data/aims/eos-si/1/inputs/control.in.gz create mode 100644 tests/test_data/aims/eos-si/1/inputs/geometry.in.gz create mode 100644 tests/test_data/aims/eos-si/1/outputs/aims.out.gz create mode 100644 tests/test_data/aims/eos-si/2/inputs/control.in.gz create mode 100644 tests/test_data/aims/eos-si/2/inputs/geometry.in.gz create mode 100644 tests/test_data/aims/eos-si/2/outputs/aims.out.gz create mode 100644 tests/test_data/aims/eos-si/3/inputs/control.in.gz create mode 100644 tests/test_data/aims/eos-si/3/inputs/geometry.in.gz create mode 100644 tests/test_data/aims/eos-si/3/outputs/aims.out.gz diff --git a/src/atomate2/aims/flows/eos.py b/src/atomate2/aims/flows/eos.py new file mode 100644 index 0000000000..ad5050c4ed --- /dev/null +++ b/src/atomate2/aims/flows/eos.py @@ -0,0 +1,82 @@ +"""Equation of state workflow for FHI-aims. Based on the common EOS workflow.""" + +from __future__ import annotations + +from dataclasses import dataclass, field +from typing import TYPE_CHECKING, Any + +from atomate2.aims.flows.core import DoubleRelaxMaker +from atomate2.aims.jobs.core import RelaxMaker +from atomate2.common.flows.eos import CommonEosMaker + +if TYPE_CHECKING: + from jobflow import Maker + + +@dataclass +class AimsEosMaker(CommonEosMaker): + """ + Generate equation of state data (based on common EOS maker). + + First relaxes a structure using initial_relax_maker, then perform a series of + deformations on the relaxed structure, and evaluate single-point energies with + static_maker. + + Parameters + ---------- + name : str + Name of the flows produced by this maker. + initial_relax_maker : .Maker | None + Maker to relax the input structure, defaults to double relaxation. + eos_relax_maker : .Maker + Maker to relax deformed structures for the EOS fit. + static_maker : .Maker | None + Maker to generate statics after each relaxation, defaults to None. + strain : tuple[float] + Percentage linear strain to apply as a deformation, default = -5% to 5%. + number_of_frames : int + Number of strain calculations to do for EOS fit, default = 6. + postprocessor : .atomate2.common.jobs.EOSPostProcessor + Optional postprocessing step, defaults to + `atomate2.common.jobs.PostProcessEosEnergy`. + _store_transformation_information : .bool = False + Whether to store the information about transformations. Unfortunately + needed at present to handle issues with emmet and pydantic validation + """ + + name: str = "aims eos" + initial_relax_maker: Maker | None = field( + default_factory=lambda: DoubleRelaxMaker.from_parameters({}) + ) + eos_relax_maker: Maker | None = field( + default_factory=lambda: RelaxMaker.fixed_cell_relaxation( + user_params={"species_dir": "tight"} + ) + ) + + @classmethod + def from_parameters(cls, parameters: dict[str, Any], **kwargs) -> AimsEosMaker: + """Creation of AimsEosMaker from parameters. + + Parameters + ---------- + parameters : dict + Dictionary of common parameters for both makers. The one exception is + `species_dir` which can be either a string or a dict with keys [`initial`, + `eos`]. If a string is given, it will be interpreted as the `species_dir` + for the `eos` Maker; the initial double relaxation will be done then with + the default `light` and `tight` species' defaults. + kwargs + Keyword arguments passed to `CommonEosMaker`. + """ + species_dir = parameters.setdefault("species_dir", "tight") + initial_params = parameters.copy() + eos_params = parameters.copy() + if isinstance(species_dir, dict): + initial_params["species_dir"] = species_dir.get("initial") + eos_params["species_dir"] = species_dir.get("eos", "tight") + return cls( + initial_relax_maker=DoubleRelaxMaker.from_parameters(initial_params), + eos_relax_maker=RelaxMaker.fixed_cell_relaxation(user_params=eos_params), + **kwargs, + ) diff --git a/tests/aims/test_flows/test_eos.py b/tests/aims/test_flows/test_eos.py new file mode 100644 index 0000000000..e35476f069 --- /dev/null +++ b/tests/aims/test_flows/test_eos.py @@ -0,0 +1,104 @@ +"""Test FHI-aims Equation of State workflow""" + +import os + +import pytest +from jobflow import run_locally +from pymatgen.core import Structure + +from atomate2.aims.flows.eos import AimsEosMaker +from atomate2.aims.jobs.core import RelaxMaker + +cwd = os.getcwd() + +# mapping from job name to directory containing test files +ref_paths = { + "Relaxation calculation 1": "double-relax-si/relax-1", + "Relaxation calculation 2": "double-relax-si/relax-2", + "Relaxation calculation (fixed cell) deformation 0": "eos-si/0", + "Relaxation calculation (fixed cell) deformation 1": "eos-si/1", + "Relaxation calculation (fixed cell) deformation 2": "eos-si/2", + "Relaxation calculation (fixed cell) deformation 3": "eos-si/3", +} + + +def test_eos(mock_aims, tmp_path, species_dir): + """A test for the equation of state flow""" + + # a relaxed structure for the test + a = 2.80791457 + si = Structure( + lattice=[[0.0, a, a], [a, 0.0, a], [a, a, 0.0]], + species=["Si", "Si"], + coords=[[0, 0, 0], [0.25, 0.25, 0.25]], + ) + + # settings passed to fake_run_aims + fake_run_kwargs = {} + + # automatically use fake AIMS + mock_aims(ref_paths, fake_run_kwargs) + + # generate flow + eos_relax_maker = RelaxMaker.fixed_cell_relaxation( + user_params={ + "species_dir": (species_dir / "light").as_posix(), + # "species_dir": "light", + "k_grid": [2, 2, 2], + } + ) + + flow = AimsEosMaker( + initial_relax_maker=None, eos_relax_maker=eos_relax_maker, number_of_frames=4 + ).make(si) + + # Run the flow or job and ensure that it finished running successfully + os.chdir(tmp_path) + responses = run_locally(flow, create_folders=True, ensure_success=True) + os.chdir(cwd) + + output = responses[flow.jobs[-1].uuid][1].output + assert "EOS" in output["relax"] + # there is no initial calculation; fit using 4 points + assert len(output["relax"]["energy"]) == 4 + assert output["relax"]["EOS"]["birch_murnaghan"]["b0"] == pytest.approx( + 0.4897486348366812 + ) + + +def test_eos_from_parameters(mock_aims, tmp_path, si, species_dir): + """A test for the equation of state flow, created from the common parameters""" + + # settings passed to fake_run_aims + fake_run_kwargs = {} + + # automatically use fake AIMS + mock_aims(ref_paths, fake_run_kwargs) + + # generate flow + flow = AimsEosMaker.from_parameters( + parameters={ + # TODO: to be changed after pymatgen PR is merged + "species_dir": { + "initial": species_dir, + "eos": (species_dir / "light").as_posix(), + }, + # "species_dir": "light", + "k_grid": [2, 2, 2], + }, + number_of_frames=4, + ).make(si) + + # Run the flow or job and ensure that it finished running successfully + os.chdir(tmp_path) + responses = run_locally(flow, create_folders=True, ensure_success=True) + os.chdir(cwd) + + output = responses[flow.jobs[-1].uuid][1].output + assert "EOS" in output["relax"] + # there is an initial calculation; fit using 5 points + assert len(output["relax"]["energy"]) == 5 + # the initial calculation also participates in the fit here + assert output["relax"]["EOS"]["birch_murnaghan"]["b0"] == pytest.approx( + 0.5189578108402951 + ) diff --git a/tests/aims/test_flows/test_phonon_workflow.py b/tests/aims/test_flows/test_phonon_workflow.py index 1270905fb9..818934d818 100644 --- a/tests/aims/test_flows/test_phonon_workflow.py +++ b/tests/aims/test_flows/test_phonon_workflow.py @@ -153,9 +153,9 @@ def test_phonon_socket_flow(si, tmp_path, mock_aims, species_dir): ) # run the flow or job and ensure that it finished running successfully - # os.chdir(tmp_path) + os.chdir(tmp_path) responses = run_locally(flow, create_folders=True, ensure_success=True) - # os.chdir(cwd) + os.chdir(cwd) # validation the outputs of the job output = responses[flow.job_uuids[-1]][1].output diff --git a/tests/test_data/aims/eos-si/0/inputs/control.in.gz b/tests/test_data/aims/eos-si/0/inputs/control.in.gz new file mode 100644 index 0000000000000000000000000000000000000000..dd999c2ecf2bcb84c451ec25afc4ff85d9e1682e GIT binary patch literal 1195 zcmV;c1XTMUiwFp>S8!$k|6^}%baHQOE@^H6wN^`S+c*%u`&SH{O9R-f-nNU~L)s!} zFN+1d=+&U5kW-JiF8MlU7&-_xyeq)~D! zo`tdEJq2!6Bg)mQ(i}|5CD&f-Wwk-opw+uUEvp-dS>zv_M(JLsZ-rfzDCLk&t6CgA ztu|Uz|4BS?ztP>TLpHj*@iU?yz~i^?Q!W|ocpDsrO#5eRx8Ow z3$>7V@2q`BFug_~xKjOE;)5@$nRuDKD$Su`xTm_$kRFKNM(6$krw{! zDWmEgZA~7QTO~^LLBDmL1GqC0#CQKJ#h%PYsx_BKm=Z!z2XN6E`HJsLiM=`F9cLbD zxH*@*!k@Efp68=Gze29ITw9HJvLf4KWp7uVvS->U%TIQ3AJm}yYM+y<3cD5Qsk-(H zaC$JNc_p}9(WD0Xf^{_%!Vu{EQ^Xc#K{{g%6im?_V2W=#NLHlXRq%jaz`TB;h?LR~{`!1eSn8hEQnqG=Y= z1ZrqVfoM9VEvKay+W^<-Y)Rqy)IuA3zaK|m2)CNHcL0&8M1$IVa@m~21I=a@g;%ow z4C2(ke^a82A00!m)LX_db$)5}9OlR;nC7#XdIL?LAFk(5(;16W_Z7-#yQ{RK!>u4= z$*Cxzq} z3$?qFQ=@gw&()9WtZ2lmFFf+2RlX2P3{0qGh J=e_t0002JNP4fT% literal 0 HcmV?d00001 diff --git a/tests/test_data/aims/eos-si/0/inputs/geometry.in.gz b/tests/test_data/aims/eos-si/0/inputs/geometry.in.gz new file mode 100644 index 0000000000000000000000000000000000000000..bdd85fb2645e206d8a30ca7aa7307fab59a053e7 GIT binary patch literal 170 zcmV;b09F4ViwFp>S8!$k|7T@yZDn+Fc`j*g0F{kP3d1lAME5y`_r*rh$Cl2K1C$WF zFr);E>G|tW+BE$^wS1a+Gmo{FDIYI+s>|7V3JTk056L+UF(&C%5v8#Mz$eztd(}N+ zWLvEd_Dyds34f^GYpY&CcKU9t%V~Y|{Ics~Fa!n#j*(OL$j)P6CN)%rrfrPeP#z8< YN@ARz2X9P7!~K2Q%&|{+cqZKH5pH~-P`B;d;dGv+E}{Rz4p1z zKEzRQa5b7v7GR&o*7h!pj&81C=f2)9YZCRBpD&oLg6hk25+N+8ooXE=)o+o$Cd1tt zORFv|_4E-T6qV9J;UxBS$*BGv-WCCU!G%9m>g*E#$p1i_Pm@$sbpLF}@7g@bfh>9J z%=DQMGE0;_e2z-(qQJ+AIcty-ZMSaXKi=#ldG{Ho-;l4o`MOr&Mp`i21U9opb6K1daMka@G76JH7S(AQ-Y|3Nj14qj7n#d zx44xIfusVQh#UA%RRALekk^0BBFt+@#B=NfpjedmnMc_{993ljaQ; 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